An international research team led by Lawrence Berkeley National Laboratory (Berkeley Lab) has taken the first atomic-resolution images and demonstrated electrical control of a chiral interface state – an exotic quantum phenomenon that could help researchers advance quantum computing and energy-efficient electronics.

The chiral interface state is a conducting channel that allows electrons to travel in only one direction, preventing them from being scattered backwards and causing energy-wasting electrical resistance. Researchers are working to better understand the properties of chiral interface states in real materials but visualizing their spatial characteristics has proved to be exceptionally difficult.

But now, for the first time, atomic-resolution images captured by a research team at Berkeley Lab and UC Berkeley have directly visualized a chiral interface state. The researchers also demonstrated on-demand creation of these resistance-free conducting channels in a 2D insulator.

Their work, which was reported in the journal Nature Physics, is part of Berkeley Lab’s broader push to advance quantum computing and other quantum information system applications, including the design and synthesis of quantum materials to address pressing technological needs.

“Our work shows for the first time what these 1D states look like at the atomic scale, including how we can alter them – and even create them.”

– Canxun Zhang, former graduate student researcher, Materials Sciences Division

“Previous experiments have demonstrated that chiral interface states exist, but no one has ever visualized them with such high resolution. Our work shows for the first time what these 1D states look like at the atomic scale, including how we can alter them – and even create them,” said first author Canxun Zhang, a former graduate student researcher in Berkeley Lab’s Materials Sciences Division and the Department of Physics at UC Berkeley. He is now a postdoctoral researcher at UC Santa Barbara.

Chiral interface states can occur in certain types of 2D materials known as quantum anomalous Hall (QAH) insulators that are insulators in bulk but conduct electrons without resistance at one-dimensional “edges” – the physical boundaries of the material and interfaces with other materials.

To prepare chiral interface states, the team worked at Berkeley Lab’s Molecular Foundry to fabricate a device called twisted monolayer-bilayer graphene, which is a stack of two atomically thin layers of graphene rotated precisely relative to one another, creating a moiré superlattice that exhibits the QAH effect.

STM images show a chiral interface state wavefunction (bright stripe) in a QAH insulator made from twisted monolayer-bilayer graphene in a 2D device. The interface can be moved across the sample by modulating the voltage on a gate electrode placed underneath the graphene layers. (Credit: Canxun Zhang/Berkeley Lab)

In subsequent experiments at the UC Berkeley Department of Physics, the researchers used a scanning tunneling microscope (STM) to detect different electronic states in the sample, allowing them to visualize the wavefunction of the chiral interface state. Other experiments showed that the chiral interface state can be moved across the sample by modulating the voltage on a gate electrode placed underneath the graphene layers. In a final demonstration of control, the researchers showed that a voltage pulse from the tip of an STM probe can “write” a chiral interface state into the sample, erase it, and even rewrite a new one where electrons flow in the opposite direction.

The findings may help researchers build tunable networks of electron channels with promise for energy-efficient microelectronics and low-power magnetic memory devices in the future, and for quantum computation making use of the exotic electron behaviors in QAH insulators.

The researchers intend to use their technique to study more exotic physics in related materials, such as anyons, a new type of quasiparticle that could enable a route to quantum computation.

“Our results provide information that wasn’t possible before. There is still a long way to go, but this is a good first step,” Zhang said.

The work was led by Michael Crommie, a senior faculty scientist in Berkeley Lab’s Materials Sciences Division and physics professor at UC Berkeley.

Tiancong Zhu, a former postdoctoral researcher in the Crommie group at Berkeley Lab and UC Berkeley, contributed as co-corresponding author and is now a physics professor at Purdue University.

The Molecular Foundry is a DOE Office of Science user facility at Berkeley Lab.

This work was supported by the DOE Office of Science. Additional funding was provided by the National Science Foundation.

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Lawrence Berkeley National Laboratory (Berkeley Lab) is committed to delivering solutions for humankind through research in clean energy, a healthy planet, and discovery science. Founded in 1931 on the belief that the biggest problems are best addressed by teams, Berkeley Lab and its scientists have been recognized with 16 Nobel Prizes. Researchers from around the world rely on the Lab’s world-class scientific facilities for their own pioneering research. Berkeley Lab is a multiprogram national laboratory managed by the University of California for the U.S. Department of Energy’s Office of Science.

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